By D. D. Eley, Herman Pines, Werner O. Haag
In view that 1948, this serial has sought to fill the distance among the papers that record and the textbooks that train within the different components of catalysis examine. The editors of and members to Advances in Catalysis are devoted to recording growth during this quarter. every one quantity of Advances in Catalysis includes articles overlaying a topic of huge curiosity.
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Extra resources for Advances in Catalysis, Vol. 40
Hatched bars are for MO, sites and dotted bars are for M 2 0 7 sites (from Ref. 39). such that it can acquire oxygen atoms up to a certain heat of reduction. In this case, as is shown in Fig. 9B, this intermediate would be able to take up a larger number of oxygen atoms from the M207 site than from the M 0 4 site. Thus the oxide with the M 2 0 7 sites would be less selective than the one with the M 0 4 sites. This example demonstrates that detailed information about the interaction of the surface intermediate with the active site is very helpful in understanding changes in selectivity patterns in oxidation catalysis.
Crystallogr. 32, IS1 (1976). 65. Atkins, P. , W. H. Freeman, New York, 1986. 66. , van Ommen, J. , and Ross, J. R. , Catul. Today 13, 629 (1992). 67. Eastman, A. , and Kimble, 1. , US Patent 4,450,313 (1984). 68. Velle, 0. J . , and Jens, K. J . , Curd. Todtcy 6, 567 (1990). 69. , and Morikawa, A , , Bull. Chem. Soc. Jpn. 63, 340 (1990). 38 HAROLD H . KUNG 70. Thorsteinson, E . , Wilson, T. , Young, F. , and Kasai, P. , J . C u r d . 52, I16 (1978). 71. , Chem. Abstr. 115; 256685 (1992). 72. , Appl.
KUNG tion selectivity, whereas ethane reacts with high dehydrogenation selectivity on (VO)2P207,but with mostly combustion on Mg3(V04)2. It became apparent that another condition is needed to explain a broader range of data, in addition to the necessary condition of possessing readily removable lattice oxygen in the active site: that the formation of oxygencontaining products be enhanced if the hydrocarbon intermediate in the selectivity-determining step can be bonded to the two vanadium ions of the linked VO, units such that the hydrocarbon species is being held close to the reactive surface lattice oxygen.
Advances in Catalysis, Vol. 40 by D. D. Eley, Herman Pines, Werner O. Haag